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This paper was realised within the framework of the Hydrogen Technology Collaboration Programme (TCP) of the International Energy Agency (IEA) in Task 40 Energy Storage and Conversion Based on Hydrogen. Some results reported in this publication were obtained thanks to funding from the Fuel Cells and Hydrogen 2 Joint Undertaking (JU) under Grant Agreement No. 826352, HyCARE project. The JU receives support from the European Union's Horizon 2020 research, Hydrogen Europe, Hydrogen Europe Research, innovation programme and Italy, France, Germany, Norway, which are all thankfully acknowledged. V A Y, R V D, M V L, S S, J B V C and M D greatly acknowledge support from EU Horizon 2020 programme in the frame of the H2020-MSCA-RISE-2017 action, HYDRIDE4MOBILITY project, with Grant Agreement 778307. J R A, J F F and F L from MIRE-group (UAM) acknowledge support from Ministerio de Ciencia, Innovacion y Universidades (RTI2018-099794-B-I100). B C H, M H S, and T R J gratefully acknowledge financial support from NordForsk Nordic Neutron Science Programme through the project FunHy (Grant Number 81942). Portions of this work were funded through the Hydrogen Materials-Advanced Research Consortium (HyMARC) of the US Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Hydrogen and Fuel Cell Technologies Office and performed under the auspices of the DOE by Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344. Additional funding for LLNL was provided through the Laboratory Directed Research and Development (LDRD) Program Project 20-SI-004. Computing resources were provided under the LLNL Institutional Computing Grand Challenge program and the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program using resources of the Argonne Leadership Computing Facility, a US Department of Energy Office of Science User Facility supported under Contract DE-AC02-06CH11357. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology and Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International, Inc., for the US Department of Energy's National Nuclear Security Administration under Contract DE-NA-0003525. The authors gratefully acknowledge funding from the US Department of Energy, Office of Energy Efficiency and Renewable Energy, Hydrogen and Fuel Cell Technologies Office, through the Hydrogen Storage Materials Advanced Research Consortium (HyMARC). This paper describes objective technical results and analysis. Any subjective views or opinions that might be expressed in the paper do not necessarily represent the views of the US Department of Energy or the United States Government. C E B, M P P, and T D H (Curtin University) acknowledge financial support from the Australian Research Council for Grants DP150101708, LE0989180 and LE0775551. T S (Shibaura Institute of Technology) acknowledges support from JST SICORP (JPMJSC 1802). S O (Tohoku University) acknowledges support from MEXT/JSPS KAKENHI 'Hydrogenomics' (JP18H05513). J-Y Suh and Y W Cho (KIST) acknowledge funding from National Research Foundation of Korea (NRF-2020M1A2A2080881). S L (University of Nottingham) acknowledges support from EPSRC (EP/V042556/1) and the use of ARCHER2 supercomputer through membership of the UK's HPC Materials Chemistry Consortium funded by EPSRC (EP/R029431/1). D B, M B, R Z S and I J (Ben Gurion University) acknowledge support from Israel Science Foundation Grant 745/15. E R wishes to thank the Grand Technion Energy Program (GTEP) for continuing support.

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Magnesium- and intermetallic alloys-based hydrides for energy storage: modelling, synthesis and properties

Publicated to:Progress in Energy. 4 (3): 032007- - 2022-07-01 4(3), DOI: 10.1088/2516-1083/ac7190

Authors: Pasquini, Luca; Sakaki, Kouji; Akiba, Etsuo; Allendorf, Mark D; Alvares, Ebert; Ares, Jose R; Babai, Dotan; Baricco, Marcello; von Colbe, Jose Bellosta; Bereznitsky, Matvey; Buckley, Craig E; Cho, Young Whan; Cuevas, Fermin; de Rango, Patricia; Dematteis, Erika Michela; Denys, Roman V; Dornheim, Martin; Fernandez, J F; Hariyadi, Arif; Hauback, Bjrn C; Heo, Tae Wook; Hirscher, Michael; Humphries, Terry D; Huot, Jacques; Jacob, Isaac; Jensen, Torben R; Jerabek, Paul; Kang, Shin Young; Keilbart, Nathan; Kim, Hyunjeong; Latroche, Michel; Leardini, F; Li, Haiwen; Ling, Sanliang; Lototskyy, Mykhaylo V; Mullen, Ryan; Orimo, Shin-ichi; Paskevicius, Mark; Pistidda, Claudio; Polanski, Marek; Puszkiel, Julian; Rabkin, Eugen; Sahlberg, Martin; Sartori, Sabrina; Santhosh, Archa; Sato, Toyoto; Shneck, Roni Z; Sorby, Magnus H; Shang, Yuanyuan; Stavila, Vitalie; Suh, Jin-Yoo; Suwarno, Suwarno; Le Thi Thu; Wan, Liwen F; Webb, Colin J; Witman, Matthew; Wan, ChuBin; Wood, Brandon C; Yartys, Volodymyr A

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Abstract

Hydrides based on magnesium and intermetallic compounds provide a viable solution to the challenge of energy storage from renewable sources, thanks to their ability to absorb and desorb hydrogen in a reversible way with a proper tuning of pressure and temperature conditions. Therefore, they are expected to play an important role in the clean energy transition and in the deployment of hydrogen as an efficient energy vector. This review, by experts of Task 40 'Energy Storage and Conversion based on Hydrogen' of the Hydrogen Technology Collaboration Programme of the International Energy Agency, reports on the latest activities of the working group 'Magnesium- and Intermetallic alloys-based Hydrides for Energy Storage'. The following topics are covered by the review: multiscale modelling of hydrides and hydrogen sorption mechanisms; synthesis and processing techniques; catalysts for hydrogen sorption in Mg; Mg-based nanostructures and new compounds; hydrides based on intermetallic TiFe alloys, high entropy alloys, Laves phases, and Pd-containing alloys. Finally, an outlook is presented on current worldwide investments and future research directions for hydrogen-based energy storage.

Keywords